The range will debut at the upmarket US retailer on May 8 and will be made available on Topshop's web site the same day.
Barneys has sold Topshop pieces previously, but this collection is expected to draw a great deal of interest because of the supermodel's international profile.
The Kate Moss Topshop collection consists of about 80 pieces and prices will range from£10 for a vest to about£200 for a soft-leather jacket.
Topshop's flagship stores will also have Kate Moss shop-in-shops.
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